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Abstract Recently, layered transition metal thiophosphate MPX₃(M= transition metals,X= S or Se) have gained significant attention because of their rich magnetic, optical, and electronic properties. Specifically, the diverse magnetic structures and the robustness of magnetism in the two-dimensional (2D) limit have made them prominent candidates to study 2D magnetism. Numerous efforts such as substitutions and interlayer intercalations have been adopted to tune the magnetic properties of these materials, which has greatly deepened the understanding of the underlying mechanisms that govern the properties. In this work, we focus on modifying the magnetism of Ising-type antiferromagnet FePS₃using electrochemical lithium intercalation. Our work demonstrate the effectiveness of electrochemical intercalation as a controllable tool to modulating magnetism, including tuning magnetic ordering temperature and inducing low temperature spin-glass state, offering an approach for implementing this material into applications. 

Abstract Observations of temporary Forbush decreases (FDs) in the Galactic cosmic-ray (GCR) flux due to the passage of solar storms are useful for space-weather studies and alerts. Here, we introduce techniques that use global networks of ground-based neutron monitors and muon detectors to measure variations of GCR rigidity spectra in space during FDs by (1) fitting count rate decreases for power-law rigidity spectra in space with anisotropy up to second order and (2) using the “leader fraction” derived from a single neutron monitor. We demonstrate that both provide consistent results for hourly spectral index variations for five major FDs, and they agree with daily space-based data when available from the Alpha Magnetic Spectrometer. We have also made the neutron monitor leader fraction publicly available in real time. This work verifies that ground-based observations can be used to precisely monitor GCR spectral variation over a wide range of rigidities during space-weather events, with results in real time or from short-term postanalysis.